![Experimental realization of bulk WS2 BIC metasurfaces. a, Sketch of the experimental process including exfoliation of WS2, nanopatterning via EBL and RIE and optical far-field spectroscopy. b, Scanning electron microscope micrographs of fabricated WS2 metasurfaces with a scaling factor of S = 1.25 with different asymmetry parameters ΔL0 and a uniform thickness of 80 nm. c, Transmittance spectra of WS2 metasurfaces (shifted for visiblility) for different ΔL0, showing the formation of the quasi-BIC modes. To show the uncoupled BIC modes, resonances were placed spectrally separated from the WS2 exciton. d, Resonance Q factors extracted from the spectra in panel c showing a maximum Q factor of 374. Credit: Nature Materials (2023). DOI: 10.1038/s41563-023-01580-7 Metasurface enables strong coupling effects between light and transition metal dichalcogenides](https://scx1.b-cdn.net/csz/news/800a/2023/metasurface-enables-st.jpg)
The interaction of light and matter on the nanoscale is a vital aspect of nanophotonics. Resonant nanosystems allow scientists to control and enhance electromagnetic energy at volumes smaller than the wavelength of the incident light. As well as allowing sunlight to be captured much more effectively, they also facilitate improved optical wave-guiding and emissions control. The strong coupling of light with electronic excitation in solid-state materials generates hybridized photonic and electronic states, so-called polaritons, which can exhibit interesting properties such as Bose-Einstein condensation and superfluidity.
A new study, published in the journal Nature Materials, presents progress in the coupling of light and matter on the nanoscale. Researchers led by LMU physicist Dr. Andreas Tittl have developed a metasurface that enables strong coupling effects between light and transition metal dichalcogenides (TMDCs). This novel platform is based on photonic bound states in the continuum, so-called BICs, in nanostructured tungsten disulfide (WS2).
The simultaneous utilization of WS2 as the base material for the manufacture of metasurfaces with sharp resonances and as a coupling partner supporting the active material excitation opens up new possibilities for research into polaritonic applications.
An important breakthrough in this research is controlling the coupling strength, which is independent of losses within the material. Because the metasurface platform is able to integrate other TMDCs or excitonic materials without difficulty, it can furnish fundamental insights and practical device concepts for polaritonic applications. Moreover, the concept of the newly developed metasurface provides a foundation for applications in controllable low-threshold semiconductor lasers, photocatalytic enhancement, and quantum computing.
More information:
Thomas Weber et al, Intrinsic strong light-matter coupling with self-hybridized bound states in the continuum in van der Waals metasurfaces, Nature Materials (2023). DOI: 10.1038/s41563-023-01580-7
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Metasurface enables strong coupling effects between light and transition metal dichalcogenides (2023, June 23)
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